| What Just Happened? (2008) | Producer |
| The Good Shepherd (2006) | Director, Producer |
| Rent (Jonathan Larson) (2005) | Producer |
| Hide & Seek (2005) | Starred as David Callaway |
| Stage Beauty (2004) | Producer |
| Godsend (2004) | Starred as Richard Wells |
| Meet The Fockers (2004) | Starred as Jack Byrnes, Producer |
| Shark Tale (2004) | Starred as Voice of Don Lino |
| About a Boy (2002) | Producer |
| City by the Sea (2002) | Starred as Detective Vincent LaMarca |
| Showtime (2002) | Starred as Mitch Preston |
| Analyze That (2002) | Starred as Paul Vitti |
| 15 Minutes (2001) | Starred as Eddie Flemming |
| The Score (2001) | Starred as Nick Wells |
| Prison Song (2001) | Producer |
| The Adventures of Rocky and Bullwinkle (2000) | Starred as Fearless Leader, Producer |
| Meet the Parents (2000) | Starred as Jack Byrnes, Producer |
| The Diver (2000) | Starred as Billy Sunday |
| Analyze This (1999) | Starred as Paul Vitti |
| Flawless (1999) | Starred as Walt Koontz |
| One Hundred and One Nights (1999) | Starred as Actor for a Day |
| Entropy (1999) | Producer |
| Great Expectations (1998) | Starred as Prisoner/Lustig |
| Ronin (1998) | Starred as Sam |
| Lenny Bruce: Swear to Tell the Truth (1998) | Narrator |
| Cop Land (1997) | Starred as Moe Tilden |
| Jackie Brown (1997) | Starred as Louis Gara |
| Wag the Dog (1997) | Starred as Conrad Brean, Producer |
| Faithful (1996) | Producer |
| The Fan (1996) | Starred as Gil Renard |
| Marvin's Room (1996) | Starred as Dr Wally, Producer |
| Sleepers (1996) | Starred as Father Bobby |
| Casino (1995) | Starred as Sam "Ace" Rothstein |
| Heat (1995) | Starred as Neil McCauley |
| Mary Shelley's Frankenstein (1994) | Starred as The Creature/Sharp Featured Man |
| A Bronx Tale (1993) | Starred as Lorenzo Anello, Director, Producer |
| Mad Dog and Glory (1993) | Starred as Wayne "Mad Dog" Dobie |
| This Boy's Life (1993) | Starred as Dwight |
| Night and the City (1992) | Starred as Harry Fabian |
| Thunderheart (1992) | Producer |
| Mistress (1992) | Starred as Evan M Wright, Producer |
| Backdraft (1991) | Starred as Donald Rimgale |
| Cape Fear (1991) | Starred as Max Cady |
| Guilty By Suspicion (1991) | Starred as David Merrill |
| Awakenings (1990) | Starred as Leonard Lowe |
| Goodfellas (1990) | Starred as James Conway |
| Stanley and Iris (1990) | Starred as Stanley Cox |
| Hollywood Mavericks (1990) | Starred as Himself |
| We're No Angels (1989) | Starred as Ned |
| Jacknife (1989) | Starred as Joseph 'Megs' Megessey |
| Midnight Run (1988) | Starred as Jack Walsh |
| Dear America: Letters Homes From Vietnam (1988) | Narrator |
| Hello Actors Studio (1988) | Starred as Himself |
| Angel Heart (1987) | Starred as Louis Cyphre |
| The Untouchables (1987) | Starred as Al Capone |
| The Mission (1986) | Starred as Captain Rodrigo Mendoza |
| Brazil (1985) | Starred as Archibald "Harry" Tuttle |
| Falling in Love (1984) | Starred as Frank Raftis |
| Once Upon a Time in America (1984) | Starred as David "Noodles" Aaronson |
| The King of Comedy (1983) | Starred as Rupert Pupkin |
| True Confessions (1981) | Starred as Des Spellacy |
| Acting: Lee Strasberg and The Actors Studio (1981) | Starred as Himself |
| Raging Bull (1980) | Starred as Jake LaMotta |
| The Deer Hunter (1978) | Starred as Michael Vronsky |
| 1900 (1977) | Starred as Alfredo Berlinghieri |
| New York, New York (1977) | Starred as Jimmy Doyle |
| The Last Tycoon (1976) | Starred as Monroe Stahr |
| The Godfather: Part II (1974) | Starred as Vito Corleone |
| Born to Win (1971) | Starred as Danny |
| The Gang That Couldn't Shoot Straight (1971) | Starred as Mario |
| Hi, Mom! (1970) | Starred as Jon Rubin |
| Bloody Mama (1970) | Starred as Lloyd Barker |
| Sam's Song (1969) | Starred as Sam |
| Greetings (1968) | Starred as Jon Rubin |
| The Wedding Party (1967) | Starred as Cecil |
| Trois Chambres a Manhattan (1965) | Starred as Bit |
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